Increasing demands on water supplies, along with concerns about non-point source pollution, and water quality–based ecological factors all point to the need for observing stream flow perturbations and pollutant discharges at higher resolution than has been practical until now. This work presents a rapidly deployable Networked Infomechanical System (NIMS RD) technology for observing spatiotemporal variability in hydraulic and chemical properties across stream channels. NIMS RD is comprised of two supporting towers and a suspension cable delivering power and Internet connectivity for controlling and actuating the tram-like NIMS unit. The NIMS unit is capable of raising and lowering a payload of sensors, allowing a preprogrammed or data-actuated adaptive scan to be completed across a stream channel. In this paper, NIMS RD is demonstrated in two relevant cases: (1) elucidating spatiotemporal variations in nutrients and other biologically significant stream constituents in Medea Creek, a small urban stream in Southern California; and (2) using high-resolution synoptic sampling of steady velocity and salinity distributions across the San Joaquin River in Central California to provide quantitative salt load estimates. For Medea Creek, temperature and specific conductivity (SC) exhibited varying cross-sectional patterns throughout each of three 24 hour scans carried out over three summer months. Both temperature and SC displayed repeating sinusoidal diel fluctuations independent of the spatial variation. For each of the months the cross-sectional variation was less during the late nighttime and morning hours than during the afternoon and early nighttime hours. For the San Joaquin River, high-resolution velocity distributions from NIMS RD were successfully reproduced in separate deployments and quantitatively matched stage-based volumetric flow rates at the site. The product of the velocity and associated SC distributions yielded total salt load estimates similar to previously reported values, but no basis for direct comparison was available.